And whenever gear ratio choices are confusing, just do the rear anyway. That way if you don't like it, you didn't just spend double to find that out.
It might not be as efficient in down-time to do one at a time, but this is a very critical moment balancing on top of that fence when deciding which way to go.
There are actually engine combinations that might like 4.11's with 33's and an overdrive, even in a Bronco. But most here are happier with 4.56's and 4.88's with that tire/transmission combo and their particular engines.
It's all about the powerband, final weight, actual tire size, how fast you drive (we know how you like to test, but how is this thing going to be driven?), what road conditions and all that, coupled with the aerodynamics (or lack thereof) of the EB.
Most of our engines won't pull well in overdrive at 2000 to 2200 rpm in a Bronco. They like 2500-2700 much better. But if your engine is a real stump-puller or just running sweet down low, you "might" be ok with 4.11. We just don't know out here other than to simply compare with what others have said. But like Broncos, every one of us is different too.
So just do the rear end first. Drive it and see how you like it and then decide what to do.
Just don't put it in 4wd until you get the front swapped over.
Paul