What is a street cruiser and light off road axle ratio for coyote swap 6r80 and 33” tires?
What gear ratio is in the Bronco now?
Whatever it is, use it at first, then decide once you've driven it. It might need lower, or it might need higher, but only you will know for sure.
And even at that point, you can still mess around, by changing only the rear 9" (if that's what you still intend to use?) gears and see how it acts on the street.
Once the happy-camper gearing is found, then you can change the front.
Unless it's been messed with, a '69 could have come from the factory with either 3.50-ish, 4.10-ish, or 4.56-ish gearing. Seemingly right in the middle of what you'd want.
But I'm thinking that for an even remotely usable overdrive, you're going to want to stay in the 4's and up (numerically speaking) to remain relevant in overdrive.
The 4.17 first gear is going to let you rocket off the line even with the 3.50 gears, but it would seem to be a dog in the upper gears. With stock 3-speed transmissions and no overdrive, 3.50's were the bane of our existence with 33 inch tires for many years.
I have 4.56 with 31" tires, which is an extreme example and totally biased towards off-road capabilities. But it's still a pleasure on the street (when it's not spinning a tire that is) with a lesser overdrive than your 6R has.
If I had to choose ahead of time (not my preference) I'd err to the side of 4.11's for your stated use.
But I'd still wait until you can drive it, then decide.
Paul